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Prog band Moon Safari can all sing so they do amazing harmonies. This short track is acapella and very nice indeed
Female Vocalists don't come much better than these two.
https://youtu.be/hL6j5LksMcM
The Aimee Mann album (she normally has nice harmonies anyway) "Mental illness has some lovely two part harmonies.
When you think of impressive, it's easy to think of multiple parts, but the ones that get me are the two part harmonies that sound big or clever.